@Article{LafrentzBKPHPYSBARB:2010:OpThSp,
author = "Lafrentz, M. and Brunne, D. and Kaminski, B. and Pavlov, V. V. and
Henriques, A. B. and Pisarev, R. V. and Yakovlev, D. R. and
Springholz, G. and Bauer, G. and Abramof, Eduardo and Rappl, P. H.
O. and Bayer, M.",
affiliation = "{Technische Universit{\"a}t Dortmund} and {Technische
Universit{\"a}t Dortmund} and {} and {Russian Academy of
Sciences} and {Johannes Kepler Universit{\"a}t Linz} and
Institute f{\"u}r Halbleiter- und Festk{\"o}rperphysik, Johannes
Kepler Universit{\"a}t Linz, 4040 Linz, Austria and {} and {} and
{Technische Universit{\"a}t Dortmund} and {Instituto Nacional de
Pesquisas Espaciais (INPE)} and {Instituto Nacional de Pesquisas
Espaciais (INPE)}",
title = "Optical third-harmonic spectroscopy of the magnetic semiconductor
EuTe",
journal = "Physical Review B",
year = "2010",
volume = "82",
number = "23",
pages = "235206",
keywords = "spectroscopy, magnetic semiconductor EuTe.",
abstract = "EuTe possesses the centrosymmetric crystal structure m3m of
rocksalt type in which the second-harmonic generation is forbidden
in electric dipole approximation but the third-harmonic generation
(THG) is allowed. We studied the THG spectra of this material and
observed several resonances in the vicinity of the band gap at
2.22.5 eV and at higher energies up to 4 eV, which are related to
four-photon THG processes. The observed resonances are assigned to
specific combinations of electronic transitions between the ground
4f7 state at the top of the valence band and excited 4f65d1 states
of Eu2+ ions, which form the lowest energy conduction band.
Temperature, magnetic field, and rotational anisotropy studies
allowed us to distinguish crystallographic and
magnetic-field-induced contributions to the THG. A strong
modification of THG intensity for the 2.4 eV band and suppression
of the THG for the 3.15 eV band was observed in applied magnetic
field. Two main features of the THG spectra were assigned to
5d(t2g) and 5d(eg) subbands at 2.4 eV and 3.15 eV, respectively. A
microscopic quantum-mechanical model of the THG response was
developed and its conclusions are in qualitative agreement with
the experimental results.",
doi = "10.1103/PhysRevB.82.235206",
url = "http://dx.doi.org/10.1103/PhysRevB.82.235206",
issn = "1098-0121",
language = "en",
targetfile = "PhysRevB.82.235206.pdf",
urlaccessdate = "02 maio 2024"
}